Difference between revisions of "Nanoparticle acoustic transducers"

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The optical sensitivity for a solid gold particle and a PS-Au core-shell particle in air are shown below (the white line is our probe wavelength):
 
The optical sensitivity for a solid gold particle and a PS-Au core-shell particle in air are shown below (the white line is our probe wavelength):
  
[[File:Sensitivity gold in air.png|500px|alt=alt text]]
+
[[File:Sensitivity gold in air.png|400px|alt=alt text]]
[[File:Sensitivity air polystyrene gold ts20nm.png|500px|alt=alt text]]
+
[[File:Sensitivity air polystyrene gold ts20nm.png|400px|alt=alt text]]
  
 
==Mechanical modelling==
 
==Mechanical modelling==
Line 31: Line 31:
  
  
[[File:Breathing mode solid particles.png |500px|alt=alt text]]
+
[[File:Breathing mode solid particles.png |400px|alt=alt text]]
[[File:Polystyrene Gold Nanoshell Air.png |500px|alt=alt text]]
+
[[File:Polystyrene Gold Nanoshell Air.png |400px|alt=alt text]]
  
 
==Experimental setup==
 
==Experimental setup==
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The experiment is based on a dual laser asynchronous optical sampling ASOPs configuration. A simple schematic of the experimental system to test the transducers is shown below:
 
The experiment is based on a dual laser asynchronous optical sampling ASOPs configuration. A simple schematic of the experimental system to test the transducers is shown below:
  
[[File: Experimental setup ASOPS.png |600px|alt=alt text]]
+
[[File: Experimental setup ASOPS.png |400px|alt=alt text]]
  
 
==Results==
 
==Results==
Line 44: Line 44:
 
Experimental measurements from 100, 125 and 150 nm solid gold particles on top of a glass are shown below. The signal contains a "coincidence peak" which occurs when the pump and probe pulses occur at the same time amd a thermal decay. These are removed by signal processing to leave just the oscillation corresponding to the mechanical response of the transducer. This is the main breathing mode frequency and is calculated by a FFT (fast fourier transform) of the oscillation.
 
Experimental measurements from 100, 125 and 150 nm solid gold particles on top of a glass are shown below. The signal contains a "coincidence peak" which occurs when the pump and probe pulses occur at the same time amd a thermal decay. These are removed by signal processing to leave just the oscillation corresponding to the mechanical response of the transducer. This is the main breathing mode frequency and is calculated by a FFT (fast fourier transform) of the oscillation.
  
[[File: Data particles.png |400px|alt=alt text]]
+
[[File: Data particles.png |300px|alt=alt text]]
  
 
==Related publications==
 
==Related publications==
 +
 +
<bibtex>
 +
@techreport{noref,
 +
title = {LU 2015 Evanston},
 +
author = {Rafael Fuentes},
 +
year = {2015},
 +
institution = {The University of Nottingham},
 +
type = {Talk},
 +
pdf = {http://optics.eee.nottingham.ac.uk/w/images/9/99/Presentation_LU2015.pdf}
 +
}
 +
</bibtex>
 +
<bibtex>
 +
@techreport{noref,
 +
title = {AFPAC 2015 Frejus},
 +
author = {Rafael Fuentes},
 +
year = {2015},
 +
institution = {The University of Nottingham},
 +
type = {Talk},
 +
pdf = {http://optics.eee.nottingham.ac.uk/w/images/d/db/Presentation_AFPAC2015.pdf}
 +
}
 +
</bibtex>
 +
 +
<bibtex>
 +
@techreport{noref,
 +
title = {Development of nanoscale ultrasonic transducers},
 +
author = {Rafael Fuentes, Richard Smith, Ferenado Perez-Cota, Sinead Tobin, Shilling Yan and Matt Clark}
 +
year = {2015},
 +
institution = {Phonons 2015, Nottingham, UK, July 2015},
 +
type = {Poster},
 +
//pdf = {http://optics.eee.nottingham.ac.uk/w/images/9/99/Poster_2011_SfB_Westminster_Nano_Transducers_RJS.pdf}
 +
}
 +
</bibtex>
 +
 +
<bibtex>
 +
@techreport{noref,
 +
title = {ultrasonic imaging with sub optical wavelength elastic waves},
 +
author = {Jon Aylot, Matt Clark, Rafael Fuentes, Leonel Marques, Fernando  Perez-Cota, Ovidio Pena-Rodriguez, Richard Smith, Sinead Tobin, Kevin  Webb}
 +
year = {2015},
 +
institution = {NINETEENTH SYMPOSIUM ON THERMOPHYSICAL PROPERTIES, Boulder, CO, USA June 21 - 26},
 +
type = {Poster},
 +
//pdf = {http://optics.eee.nottingham.ac.uk/w/images/9/99/Poster_2011_SfB_Westminster_Nano_Transducers_RJS.pdf}
 +
}
 +
</bibtex>

Latest revision as of 13:36, 11 March 2016

Introduction

There has been much interest in the optical and mechanical properties of solid and core-shell nanoparticles. Our interest stems from the ability of such devices to interact with ultrasound of very short wavelength allowing the possibility of high resolution acoustic imaging.

There are a number of different fabrication approaches that could be adopted for making nano ultrasonic transducers. Previously, a plate transducer for cell imaging has been developed, but making the lateral dimensions of the transducer smaller than one micron is challenging. An alternative approach to overcome this difficulty and to increase the frequency is to make transducers using nanoparticles.

Nanoparticle acoustic transducers have some attractions:

  • Small size
  • Can be made in large quantities
  • Easy symmetry
  • Can exploit plasmonics to enhance the detection sensitivity (for metal particles)

Optical modelling

The optical sensitivity of the transducer is governed by Mie scattering. The layer structure is designed so that the metal layer is partial reflector. Part of the probe beam incident on the transducer is transmitted into the cavity and is resonantly reflected (and transmitted) by the structure. The transducer (when it vibrates) has to show a high optical sensitivity for the probe wavelength (780 nm) in transmission or/and reflection.

The scattering and backscattering efficiencies are obtained:

alt text

where each layer is characterised by the size parameter xL=2πNrl and the relative refractive index ml=nl/nm, where λ is the wavelength of the incident wave in vacuum, rl is the outer radius of the lth layer, nm and nl are the refractive index of the medium outside the particle of its lth component, respectively, and k is the propagation constant.

The optical sensitivity for a solid gold particle and a PS-Au core-shell particle in air are shown below (the white line is our probe wavelength):

alt text alt text

Mechanical modelling

In order to make our transducers resonate at a specific frequency, the main breathing mode frequency has to be modelled based on the parameters of the transducer.

The main breathing mode for a solid silica/gold/polystyrene particle and PS-Au core-shell particle in air are shown below:


alt text alt text

Experimental setup

The experiment is based on a dual laser asynchronous optical sampling ASOPs configuration. A simple schematic of the experimental system to test the transducers is shown below:

alt text

Results

Experimental measurements from 100, 125 and 150 nm solid gold particles on top of a glass are shown below. The signal contains a "coincidence peak" which occurs when the pump and probe pulses occur at the same time amd a thermal decay. These are removed by signal processing to leave just the oscillation corresponding to the mechanical response of the transducer. This is the main breathing mode frequency and is calculated by a FFT (fast fourier transform) of the oscillation.

alt text

Related publications

Rafael Fuentes - LU 2015 Evanston
Technical Report - Talk, The University of Nottingham ,2015
Bibtex
Author : Rafael Fuentes
Title : LU 2015 Evanston
In : Technical Report - Talk, The University of Nottingham -
Address :
Date : 2015

Rafael Fuentes - AFPAC 2015 Frejus
Technical Report - Talk, The University of Nottingham ,2015
Bibtex
Author : Rafael Fuentes
Title : AFPAC 2015 Frejus
In : Technical Report - Talk, The University of Nottingham -
Address :
Date : 2015

Rafael Fuentes, Richard Smith, Ferenado Perez-Cota, Sinead Tobin, Shilling Yan, Matt Clark - Development of nanoscale ultrasonic transducers
Technical Report - Poster, Phonons 2015, Nottingham, UK, July 2015 ,2015
Bibtex
Author : Rafael Fuentes, Richard Smith, Ferenado Perez-Cota, Sinead Tobin, Shilling Yan, Matt Clark
Title : Development of nanoscale ultrasonic transducers
In : Technical Report - Poster, Phonons 2015, Nottingham, UK, July 2015 -
Address :
Date : 2015

Jon Aylot, Matt Clark, Rafael Fuentes, Leonel Marques, Fernando Perez-Cota, Ovidio Pena-Rodriguez, Richard Smith, Sinead Tobin, Kevin Webb - ultrasonic imaging with sub optical wavelength elastic waves
Technical Report - Poster, NINETEENTH SYMPOSIUM ON THERMOPHYSICAL PROPERTIES, Boulder, CO, USA June 21 - 26 ,2015
Bibtex
Author : Jon Aylot, Matt Clark, Rafael Fuentes, Leonel Marques, Fernando Perez-Cota, Ovidio Pena-Rodriguez, Richard Smith, Sinead Tobin, Kevin Webb
Title : ultrasonic imaging with sub optical wavelength elastic waves
In : Technical Report - Poster, NINETEENTH SYMPOSIUM ON THERMOPHYSICAL PROPERTIES, Boulder, CO, USA June 21 - 26 -
Address :
Date : 2015